Dissolved organic matter in surface runoff in the Loess Plateau of China: The role of rainfall events and land-use     

Zhongwu Li  Hao Peng  Binggeng Xie  Chun Liu  Xiaodong Nie  Danyang Wang  Mei Huang  Haibing Xiao  Lin Shi  Xuqin Zhang  Jieyu Jiang 《水文研究》2020,34(6):1446-1459

Exploring the chemical characterization of dissolved organic matter (DOM) is important for understanding the fate of laterally transported organic matter in watersheds. We hypothesized that differences in water-extractable organic matter (WEOM) in soils of varying land uses and rainfall events may significantly affect the quality and the quantity of stream DOM. To test our hypotheses, characteristics of rainfall-runoff DOM and WEOM of source materials (topsoil from different land uses and gullies, as well as typical vegetation) were investigated at two adjacent catchments in the Loess Plateau of China, using ultraviolet–visible absorbance and excitation emission matrix fluorescence with parallel factor analysis (PARAFAC). Results indicated that land-use types may significantly affect the chemical composition of soil WEOM, including its aromaticity, molecular weight, and degree of humification. The PARAFAC analysis demonstrated that the soils and stream water were dominated by terrestrial/allochthonous humic-like substances and microbial transformable humic-like fluorophores. Shifts in the fluorescence properties of stream DOM suggested a pronounced change in the relative proportion of allochthonous versus autochthonous material under different rainfall patterns and land uses. For example, high proportions of forestland could provide more allochthonous DOM input. This study highlights the relevance of soils and hydrological dynamics on the composition and fluxes of DOM issuing from watersheds. The composition of DOM in soils was influenced by land-use type. Precipitation patterns influenced the proportion of terrestrial versus microbial origins of DOM in surface runoff. Contributions of allochthonous, terrestrially derived DOM inputs were highest from forested landscapes.  相似文献   

A method for evaluating the longitudinal functional connectivity of a river–lake–marsh system and its application in China     

Yeling Liu  Baoshan Cui  Jizeng Du  Qing Wang  Shuling Yu  Wei Yang 《水文研究》2020,34(26):5278-5297

The longitudinal functional connectivity of a river–lake–marsh system (RLMS) refers to the actual water-mediated transport of material from upstream to downstream areas along a spatial gradient and is fundamental to understand hydrological and biogeochemical cycles. However, due to a lack of consensus on appropriate data and methods, the quantification of connectivity is still a challenge, especially at the catchment scale. We developed a new method to evaluate longitudinal functional connectivity based on fluxes of materials (water, sediment, and chemicals) along a RLMS. The calculation of fluxes is based on the longitudinal pattern of terrain gradient, which influences transport efficiency, and on contributions from hillslopes, which set the initial spatial template of material loading to the RLMS. We evaluate the contributions from hillslopes to RLMS based on a new modified version of the index of sediment connectivity (IC) proposed by Borselli et al. (2008) and revised by Chartin et al. (2017).We applied this method to the Baiyangdian Basin covering an area of 3.4 × 10⁴ km² in China and quantified longitudinal functional connectivity during normal, wet, and dry periods(April, July and December) in year 2016. We found that areas with good structural connectivity exhibited poor functional connectivity during the normal and dry periods. Modelling testing with discharge data from hydrological stations and measured chemicals from Baiyangdian Lake was satisfactory in test periods. We conclude that public data and Digital Elevation Model-derived information can be used to reliably map the longitudinal functional connectivity of RLMSs. The proposed method provides a useful tool for monitoring and restoring the longitudinal functional connectivity of RLMSs and our results indicate that efforts aimed at restoring functional connectivity in RLMSs should take into account landscape patterns that can greatly influence fluxes in the watershed.  相似文献   

How soil texture,channel shape and cross-sectional area affect moisture dynamics and water loss in irrigation channels     

Zhifan Mu  Tianxiao Li  Dong Liu  Qiang Fu  Renjie Hou  Qinglin Li  Yi Ji  Song Cui  Mo Li 《水文研究》2021,35(4):e14155

To enhance the utilization efficiency of farmland irrigation water and reduce the leakage of water conveyance channels, the leakage process of channels was simulated dynamically. The simulated results were compared with data measured in laboratory experiments, and the performance of the model was evaluated. The results indicated that the simulated values of the model were consistent with the observation values, and the R² values varied between 0.91 and 0.99. In addition, based on the laboratory experiments, a water supply system (Mariotte bottles) and soil box were built using plexiglass. Three influencing factors, namely, the channel form, soil texture and channel cross-sectional area, were varied to observe and calculate the resulting cumulative infiltration amount, infiltration rate and wetting front migration distance. HYDRUS-3D software was used to solve the three-dimensional soil water movement equation under different initial conditions. The results demonstrated that the U-shaped channel was more effective than the trapezoidal channel in increasing the utilization efficiency of the water resources. A U-shaped channel with a small channel cross-sectional area should be adopted and the soil particle size should be prioritized in the construction of water conveyance channels for farmlands. The simulation results were in agreement with the observed results, which indicates that HYDRUS-3D is a reliable tool that can accurately simulate the soil moisture movement in water conveyance channels. The research results can provide a reference for the design and operation of farmland irrigation systems.  相似文献   

Response of soil aggregate disintegration to the different content of organic carbon and its fractions during splash erosion     

Hairu Li  Gang Liu  Ju Gu  Hong Chen  Hongqiang Shi  Mohamed A. M. Abd Elbasit  Feinan Hu 《水文研究》2021,35(2):e14060

Aggregate disintegration is a critical process in soil splash erosion. However, the effect of soil organic carbon (SOC) and its fractions on soil aggregates disintegration is still not clear. In this study, five soils with similar clay contents and different contents of SOC have been used. The effects of slaking and mechanical striking on splash erosion were distinguished by using deionized water and 95% ethanol as raindrops. The simulated rainfall experiments were carried out in four heights (0.5, 1.0, 1.5 and 2.0 m). The result indicated that the soil aggregate stability increased with the increases of SOC and light fraction organic carbon (LFOC). The relative slaking and the mechanical striking index increased with the decreases of SOC and LFOC. The reduction of macroaggregates in eroded soil gradually decreased with the increase of SOC and LFOC, especially in alcohol test. The amount of macroaggregates (>0.25 mm) in deionized water tests were significantly less than that in alcohol tests under the same rainfall heights. The contribution of slaking to splash erosion increased with the decrease of heavy fractions organic carbon. The contribution of mechanical striking was dominant when the rainfall kinetic energy increased to a range of threshold between 9 J m⁻² mm⁻¹ and 12 m⁻² mm⁻¹. This study could provide the scientific basis for deeply understanding the mechanism of soil aggregates disintegration and splash erosion.  相似文献   

微塑料对海洋桡足类摄食、排泄及生殖的影响     

于娟  许瑞  魏逾杰  田继远  王雪丹  来敬广  陈容  杨桂朋  张正雨  邵云粹 《中国海洋大学学报(自然科学版)》2020,50(3):73-80

微塑料污染目前成为海洋污染普遍关注的一个研究热点。本文在实验室内将青岛近海常见的海洋桡足类猛水蚤暴露于不同浓度的微塑料尼龙6中,研究了猛水蚤的摄食、排泄以及生殖的变化。研究结果表明,微塑料尼龙6对猛水蚤的摄食、排泄、生殖均产生不利的影响,并且存在剂量-效应关系。微塑料尼龙6对猛水蚤摄食率、滤水率、排粪率的24 h·EC 50分别为67.7、62.2、84.1 mg·L^-1,对猛水蚤抱卵率的144 h·EC 50为30.3 mg·L^-1。“饱食感”造成猛水蚤摄食率降低,从而能量和营养摄入不足可能是导致猛水蚤抱卵率降低的原因。猛水蚤对微塑料的摄食,导致猛水蚤排泄的粪便颗粒小型化,由长椭球体变为短小椭球体,可能与其粘度或物理结构的改变有关。暴露于尼龙6的猛水蚤的粪便体积和沉降速率显著低于未暴露微塑料的对照组。本实验结果对于研究微塑料对海洋桡足类以及滤食性浮游动物的生态毒理影响具有一定的帮助。  相似文献   

Adding the missing third and fourth dimensions to trajectory analysis in carbonate systems     

Philipp Tesch  Robert S. Reece  James R. Markello  Juan Carlos Laya  Michael C. Pope 《Basin Research》2020,32(2):388-401

We developed a seismic geomorphology-based procedure to enhance traditional trajectory analysis with the ability to visualize and quantify lateral variability along carbonate prograding-margin types (ramps and rimmed shelves) in 3D and 4D. This quantitative approach analysed the shelf break geometric evolution of the Oligo-Miocene carbonate clinoform system in the Browse Basin and delineated the feedback between antecedent topography and carbonate system response as controlling factor on shelf break rugosity. Our geometrical analysis identified a systematic shift in the large-scale average shelf break strike direction over a transect of 10 km from 62° to 55° in the Oligo-Miocene interval of the Browse Basin, which is likely controlled by far-field allogenic forcing from the Timor Trough collision zone. Plotting of 3D shelf break trajectories represents a convenient way to visualize the lateral variability in shelf break evolution. Shelf break trajectories that indicate contemporaneous along-strike progradation and retrogradation correlate with phases of autogenic slope system re-organization and may be a proxy for morphological stability of the shelf break. Shelf break rugosity and shelf break trajectory rugosity are not inherited parameters and antecedent topography does not dictate long-term differential movement of the shelf margin through successive depositional sequences. The autogenic carbonate system response to antecedent topography smooths high-rugosity areas by filling accommodation and maintains a relatively constant shelf break rugosity of ~150 m. Color-coding of the vertical component in the shelf break trajectory captures the creation and filling of accommodation, and highlights areas of the transect that are likely to yield inconsistent 2D sequence stratigraphic interpretations.  相似文献   

华北克拉通南缘石炭系本溪组铁-铝黏土矿物质来源: 以河南三门峡大安铝黏土矿床为例^*          下载免费PDF全文

刘学飞  王庆飞  马遥  李中明  赵利华  周智慧  刘百顺  马欣莉 《古地理学报》2020,22(5):965-976

华北克拉通在中奥陶世至晚石炭世期间一直出露地表,经历了长期的风化作用,形成大规模的铁-铝黏土矿,其成矿物源一直是研究的热点,尤其是本溪组底部铁矿和铁质黏土矿与上部铝黏土矿是否为同一来源尚未查清。本研究选取克拉通南缘大安铝黏土矿床作为研究对象,展开微区矿物及元素地球化学组成分析,进一步探讨铁-铝黏土矿物质来源。大安矿床内含矿岩系自下而上包括铁质黏土岩、铝土矿、铝质黏土矿;局部喀斯特高地缺失铝土矿,铝质黏土矿直接覆盖于铁质黏土岩之上。铁质黏土岩在洼地以菱铁矿、黄铁矿和伊利石为主,在隆起区以赤铁矿、伊利石和高岭石为主。铝土矿以硬水铝石、伊利石和锐钛矿为主;铝质黏土矿主要矿物为伊利石。矿物微区分析在黏土矿底部发现大量的碳化硅和少量自然硅、硅铁矿、铬铁矿;区域对比揭示北秦岭造山带内商丹缝合带和二郎坪群中的蛇绿岩为铝黏土矿形成提供了成矿物质。本溪组底部铁质黏土与上部铝黏土矿稳定元素比率(例如Zr/TiO₂、Hf/TiO₂、Nb/TiO₂、Ta/TiO₂)存在明显差异,揭示二者为不同来源: 底部铁质黏土岩和铁矿层为底板碳酸盐岩原地风化的产物;而上部铝黏土矿是异地搬运物,北秦岭造山带在晚石炭世的整体抬升为华北铝黏土矿形成提供了重要的成矿物质。  相似文献   

Mineralogy,Fluid Inclusion,and Hydrogen and Oxygen Isotope Studies of the Intrusion‐Related Yangla Cu Deposit in the Sanjiang Region,SW China: Implications for Metallogenesis and Deposit Type     

Li‐Juan Du  Bo Li  Zhi‐Long Huang  Jun Chen  Jia‐Xi Zhou  Guo‐Fu Zou  Zai‐Fei Yan 《Resource Geology》2020,70(1):28-49

The Yangla deposit is an intrusion‐related Cu deposit in the Jinshajiang tectonic belt (eastern Sanjiang region, SW China). Despite extensive studies that have been conducted on this deposit, the relationship between the granitic magma and Cu mineralization is still unclear, and hence, the genesis is debated. To answer this question, we conducted an integrated study of mineralogy, fluid inclusions (FIs), and hydrogen and oxygen (H‐O) isotopes. Three mineralization stages were identified based on the ore textures, alteration zonation, and crosscutting relationships: (i) pre‐ore prograde skarn (stage I), with the garnet and pyroxene dominated by andradite and diopside, respectively; (ii) syn‐ore retrograde alteration (stage II), which is subdivided into the early syn‐ore stage (stage IIa) marked by retrograde hydrated mineral assemblages and significant Fe‐Cu‐Mo‐Pb‐Zn sulfide mineralization, and the late syn‐ore stage (stage IIb) featured by quartz‐calcite veins; and (iii) late supergene mineralization (stage III), which is characterized by secondary azurite and malachite. These results of mineralogy, FIs, and H‐O isotopes indicate that: (i) Cu mineralization has a close temporal, spatial, and genetic relationship with skarn alteration; (ii) the ore fluids were magmatic dominated with late‐stage meteoric water incursion; and (iii) Type‐S (halite‐bearing) and Type‐V (vapor‐rich) FIs coexisted in garnet and clinopyroxene of stage I, indicating that fluid boiling might have occurred during this stage. From stage I to stage IIa, the FI type transformed from Type‐S + Type‐V + Type‐L (liquid‐rich) to Type‐V + Type‐L with the conduct of mineralization and was accompanied by the disappearance of Type‐S, and homogenization temperature and salinity also tended to decrease dramatically, which may be caused by the deposition of skarn minerals. At stage IIa, boiling of the ore fluids still continued due to the change from lithostatic to hydrostatic pressure, which triggered the precipitation of abundant quartz‐Cu‐Mo‐Fe sulfides. Furthermore, fluid mixing between a high‐temperature magmatic fluid and a low‐temperature meteoric water might cause a considerable drop in temperature and the deposition of Cu‐bearing quartz/calcite veins during stage IIb. Hence, we consider the Yangla deposit to be of a skarn type, genetically related to the Mesozoic magmatism in the Sanjiang region.  相似文献   

浊积岩和砂质碎屑流岩关键识别标志及辽河盆地岩心实例^*          下载免费PDF全文

杨棵  朱筱敏  刘宇  刘兴周  郭峰 《古地理学报》2020,22(3):483-492

重力流是自然界中广泛存在的一种流体形式,不同学者基于不同切入点往往会提出多种重力流的划分方案。采用浊流和碎屑流的二分方案,对浊积岩和砂质碎屑流岩的沉积特征展开综述和探讨,旨在进一步概括这2类岩石的沉积特征,明确具有指示意义的最典型相标志。研究表明,在野外露头和钻井岩心中,可以通过以下典型特征鉴别浊积岩和砂质碎屑流岩: 砂岩内若发育以正粒序为特征的递变层理,则应该将其认定为浊积岩;若砂岩内发育泥岩撕裂屑、漂浮状泥砾或不含任何层理构造(块状砂岩),则应该将其认定为砂质碎屑流岩。这些特征是鉴别浊积岩和砂质碎屑流岩最可靠的标志。此外,变形层理、爬升波纹交错层理、波状层理、平行纹层、冲刷侵蚀界面、岩性突变界面和槽模等沉积构造也具有一定指示意义,出现这些特征时需要结合沉积背景、岩相的垂向组合关系和地球物理等资料进行综合判断。  相似文献   

渤海湾盆地歧口凹陷地层压力结构特征     

姜文亚  宋泽章  周立宏  蒲秀刚  王娜  代昆  万伟超  刘祥柏 《吉林大学学报(地球科学版)》2020,50(1):52-69

深化含油气沉积盆地的压力结构研究，厘清异常压力的空间展布，对划分含油气系统、评价有利输导体系与明确勘探甜点区带具有重要的理论和实践意义。为深化渤海湾盆地富油凹陷的油气二次勘探，本文以歧口凹陷为研究对象，对其压力结构进行重点刻画。在实测地层压力的校正下，综合单井、连井和二维地震地层压力结构分析，厘清了歧口凹陷的压力结构特征，识别出4类纵向压力结构：①单超压带结构；②双超压带结构；③多超压带结构；④静水压力结构。纵向上，歧口地区存在3类纵向压力系统样式——单超压系统、双超压系统、静水常压系统。双超压系统是歧口凹陷的主要压力系统样式，广泛发育于主凹和各大次凹；从凹陷中心向盆地边缘，双超压系统逐渐向单超压系统、静水常压系统过渡。单超压系统主要分布于盆地边缘的斜坡和潜山区，如歧北高斜坡、羊三木-扣村潜山等。静水常压系统则主要分布在离深凹区更远的沈青庄潜山和埕北斜坡区域。上部超压系统和下部超压系统的顶板分别位于东营组和沙三段内部，侧向上受盆地边缘和深大断裂控制。上部超压系统的形成主要受欠压实作用控制，以歧口主凹为中心呈环带分布；而下部超压系统的形成主要受生烃作用控制，以主凹和几大次凹为中心分布。未来，下部超压系统中保存的天然气将成为歧口地区超深层天然气勘探的重点对象。  相似文献